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If you have a post bound album, which usually has a rounded spine it can be a little difficult to write something on the spine. You could either stick a decorated label on the spine (using labels that are memory-safe) or write carefully with some fabric paint (assuming you have a fabric album). For leather albums you could find a small photo pocket to stick on the spine and then slip a card with your label.
When labeling the albums you want to make sure you do something subtle and neat so you don't ruin your album.